It's very difficult to find organizations these days to accept your used toys. Here is a shortlist of organizations that will accept your toys and other donated items.
Donate your used toys and children's clothing to:
Big Brothers Big Sisters of Long Island
Donation Line: (631) 234-0000
http://www.bbbsli.org/
Accepts children's clothing (all sizes), toys - games/tools, bedding, and other items.
Vietnam Veterans of America
Donation Line: (631) 582-0242
http://www.wepickup.org/
Accepts toys, small furniture, and other items.
Lupus Foundation of America, Inc.
Donation Line: (888) 445-8787
http://www.lupuspickup.org/
Accepts toys - games, clothing, bedding, and other items.